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This is a process to bypass a lot of the complexity of making plaster moulds for slipcasting or press moulding. It might be possible to press the clay directly into the silicone, but the silicone is flexible and won't absorb moisture. These will be quite limiting compared to plaster.
Overall, this is a moderately complicated project, but is easier and will hopefully give better results than most introductions to plaster!
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Link to tools: www.oldforgecreations.co.uk/r...